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巻内 崇彦*; 日置 友智*; 清水 祐樹*; 星 幸治郎*; Elyasi, M.*; 山本 慧; 横井 直人*; Serga, A. A.*; Hillebrands, B.*; Bauer, G. E. W.*; et al.
Nature Materials, 23(5), p.627 - 632, 2024/05
When excited, a magnetization in a magnet precesses around the field in an anticlockwise manner on a time scale governed by viscous magnetization damping, after which any information carried by the initial actuation seems to be lost. The damping appears to be a fundamental bottleneck for the use of magnets in information processing. Nevertheless, here we demonstrate recall of the magnetization-precession phase after times that far exceed the damping time scale by two orders of magnitude using dedicated two-colour microwave pump-and-probe experiments for a Y
Fe
O
microstructured film. Time- resolved magnetization state tomography confirms the magnetic persistent coherence (MPC) by revealing a double-exponential decay of the magnetization correlation. We attribute MPC to a feedback effect, viz. coherent coupling of the uniform precession with long-lived excitations at the minima of the spin-wave dispersion relation. Our finding liberates magnetic systems from the strong damping in nanostructures tyranny that limits their use in coherent information storage and processing.
山本 慧
JPSJ News and Comments (Internet), 21, p.07_1 - 07_2, 2024/04
A novel mechanism for generating net magnetization from phonons in chiral crystals builds upon the modern notion of geometric phases and extends the scope of century-old research efforts to understand the transfer of angular momentum between lattice and spins.
Co, Ni, and 
Co and the influence of the 
orbitalAjayi, S.*; Tripathi, V.*; Rubino, E.*; Bhattacharya, S.*; Baby, L. T.*; Lubna, R. S.*; Benetti, C.*; Wibisono, C.*; Wheeler, M. B.*; Tabor, S. L.*; et al.
Physical Review C, 109(1), p.014305_1 - 014305_21, 2024/01
被引用回数：0 パーセンタイル：0.19(Physics, Nuclear)フロリダ州立大学のタンデム加速器にてCo, NiとCoの励起状態を生成し、そこからの脱励起ガンマ線からエネルギー準位を得た。Coについては
までの、Niについては
までの高スピン状態が得られた。これらの結果を
殻から-
軌道に1個までの励起を許す大規模殻模型計算と比較した結果、スピンがかなり大きなもの以外のイラスト状態の励起エネルギーをよく再現した。再現できなかった高スピン状態は、多粒子多空孔励起が主であると考えられる。また、殻模型計算からは、これらの高スピン状態のいくつかは
遷移強度が強いバンドと考えられる。
古府 麻衣子; 河村 聖子; 村井 直樹; 石井 梨恵子*; 平井 大悟郎*; 有馬 寛*; 舟越 賢一*
Physical Review Research (Internet), 6(1), p.013006_1 - 013006_9, 2024/01
We revisited spin dynamics in archetypical classical spin glass systems, such as Cu
Mn
(
, 0.034, and 0.067) dilute alloys and iron aluminosilicate glass using a modern neutron scattering spectrometer with high neutron flux. The former is crystalline, and the latter is amorphous, where their spin glass state is well separated from magnetically ordered phases. Bose-scaled localized magnetic excitations were observed in both compounds below the spin-freezing temperature (
). The spectrum exhibits a maximum at low energy and a broad tail on the high-energy side. The excitation energy tends to be higher for the material with a higher . Above the , the spectrum considerably changes with temperature, thereby indicating the emergence of the magnetic relaxation process. The magnetic excitation in the spin glass state has much in common with the boson peak in structural glasses. We consider that the Bose-scaled broad excitation peak is an elementary excitation inherent in disordered systems.
徳永 陽; 酒井 宏典; 神戸 振作; Opletal, P.; 常盤 欣文; 芳賀 芳範; 北川 俊作*; 石田 憲二*; 青木 大*; Knebel, G.*; et al.
Physical Review Letters, 131(22), p.226503_1 - 226503_7, 2023/12
被引用回数：0 パーセンタイル：0(Physics, Multidisciplinary)Our measurements of 
Te NMR relaxations reveal an enhancement of electronic spin fluctuations above 
~T, leading to their divergence in the vicinity of the metamagnetic transition at 
~T, below which field-reinforced superconductivity appears when a magnetic field (
) is applied along the crystallographic 
axis. The NMR data evidence that these fluctuations are dominantly longitudinal, providing a key to understanding the peculiar superconducting phase diagram in 
, where such fluctuations enhance the pairing interactions.
森 道康; Ziman, T.*
IEEE Transactions on Magnetics, 59(11), p.1300505_1 - 1300505_5, 2023/11
被引用回数：0 パーセンタイル：0(Engineering, Electrical & Electronic)We introduce a simple model for the ferrimagnetic non-collinear "magnetic umbrella" states of rare-earth iron garnets (REIG), common when the rare-earth moments have non-zero orbital angular momentum. The spin-wave excitations are calculated within linear spin wave theory and temperature effects via mean-field theory. By the symmetry of the model, only one rare earth mode hybridizes, inducing a gap at zero wave number and level repulsion at finite frequency. At the compensation point, the hybridization gap closes and finally, as we approach the N
el temperature, the hybridization gap appears to reopen. The chirality of the lowest mode changes its sign around the frequency at which the level repulsion occurs. This is important to estimate the spin current generation in REIGs.
Lyons, T. P.*; Puebla, J.*; 山本 慧; Deacon, R. S.*; Hwang, Y.*; 石橋 幸治*; 前川 禎通*; 大谷 義近*
Physical Review Letters, 131(19), p.196701_1 - 196701_6, 2023/11
被引用回数：2 パーセンタイル：0(Physics, Multidisciplinary)Harnessing the causal relationships between mechanical and magnetic properties of van der Waals materials presents a wealth of untapped opportunity for scientific and technological advancement, from precision sensing to novel memories. This can, however, only be exploited if the means exist to efficiently interface with the magnetoelastic interaction. Here, we demonstrate acoustically-driven spin-wave resonance in a crystalline antiferromagnet, chromium trichloride, via surface acoustic wave irradiation. The resulting magnon-phonon coupling is found to depend strongly on sample temperature and external magnetic field orientation, and displays a high sensitivity to extremely weak magnetic anisotropy fields in the few mT range. Our work demonstrates a natural pairing between power-efficient strain-wave technology and the excellent mechanical properties of van der Waals materials, representing a foothold towards widespread future adoption of dynamic magneto-acoustics.
Liao, L.*; Puebla, J.*; 山本 慧; Kim, J.*; 前川 禎通*; Hwang, Y.*; Ba, Y.*; 大谷 義近*
Physical Review Letters, 131(17), p.176701_1 - 176701_6, 2023/10
被引用回数：2 パーセンタイル：0(Physics, Multidisciplinary)Phonons and magnons are engineered by periodic potential landscapes in phononic and magnonic crystals, and their combined studies may enable valley phonon transport tunable by the magnetic field. Through nonreciprocal surface acoustic wave transmission, we demonstrate valley-selective phonon-magnon scattering in magnetoelastic superlattices. The lattice symmetry and the out-of-plane magnetization component control the sign of nonreciprocity. The phonons in the valleys play a crucial role in generating nonreciprocal transmission by inducing helical strains that couple with the magnons. The transmission spectra show a nonreciprocity peak near a transmission gap, matching the phononic band structure. Our results open the way for manipulating valley phonon transport through periodically varying magnon-phonon coupling.
金城 克樹*; 藤林 裕己*; 松村 拓輝*; 堀 文哉*; 北川 俊作*; 石田 憲二*; 徳永 陽; 酒井 宏典; 神戸 振作; 仲村 愛*; et al.
Science Advances (Internet), 9(30), p.2736_1 - 2736_6, 2023/07
被引用回数：0 パーセンタイル：0(Multidisciplinary Sciences)Superconducting (SC) state has spin and orbital degrees of freedom, and spin-triplet superconductivity shows multiple SC phases because of the presence of these degrees of freedom. However, the observation of spin-direction rotation occurring inside the SC state (SC spin rotation) has hardly been reported. Uranium ditelluride, a recently found topological superconductor, exhibits various SC phases under pressure: SC state at ambient pressure (SC1), high-temperature SC state above 0.5 gigapascal (SC2), and low-temperature SC state above 0.5 gigapascal (SC3). We performed nuclear magnetic resonance (NMR) and ac susceptibility measurements on a single-crystal uranium ditelluride. The b axis spin susceptibility remains unchanged in SC2, unlike in SC1, and decreases below the SC2-SC3 transition with spin modulation. These unique properties in SC3 arise from the coexistence of two SC order parameters. Our NMR results confirm spin-triplet superconductivity with SC spin parallel to b axis in SC2 and unveil the remaining of spin degrees of freedom in SC uranium ditelluride.
山野井 一人*; 榊原 有理*; 藤本 純治*; 松尾 衛; 能崎 幸雄*
Applied Physics Express, 16(6), p.063004_1 - 063004_6, 2023/06
被引用回数：0 パーセンタイル：0(Physics, Applied)We report a large modulation of spin pumping using temperature-induced magnetic phase transitions in c-axis oriented single crystalline dysprosium (Dy). From the temperature variation of the magnetic susceptibility, transitions from paramagnetic (PM) to ferromagnetic (FM) phases via antiferromagnetic (AFM) phase are clearly observed in the Dy. Unlike polycrystalline Dy, the spin pumping of both PM- and AFM-Dy are strongly suppressed owing to the increased non-dissipative backflow of spin current by the long-range spin transport, although two orders of magnitude difference exist between FM- and AFM-phases.
荒木 康史; 家田 淳一
Journal of the Physical Society of Japan, 92(7), p.074705_1 - 074705_9, 2023/06
被引用回数：0 パーセンタイル：0(Physics, Multidisciplinary)トポロジカル絶縁体は電子が波数空間でトポロジカル構造を持つことにより、様々な非自明な電磁応答現象を示す。一方で、現在用いられているインダクタ・キャパシタの動作原理は、マクスウェル方程式によって記述される古典電磁気学に基づいている。本研究では絶縁体中のトポロジカル電磁応答が、磁性体中の磁化ダイナミクスと組み合わさることにより、インダクタンス・キャパシタンスを生み出すことを示す。まず、トポロジカル場の理論に基づいて、複素インピーダンスを導出する理論的枠組みを提案する。次にその理論に基づき、接合系のセットアップでインダクタンス・キャパシタンスが発現することを示す。金属磁性体における創発インダクタンスに関する先行研究と比較すると、トポロジカル絶縁体はジュール熱を抑制できるため、素子内での電力損失を大幅に抑制することができる。これによって、トポロジカル電磁応答に起因したインダクタンスは弱電流・高周波数での動作を可能とし、更に電力効率の面でも高い品質係数(Q値)を実現できることを示す。
Te-NMR on the uranium-based superconductor UTe藤林 裕己*; 金城 克樹*; 仲嶺 元輝*; 北川 俊作*; 石田 憲二*; 徳永 陽; 酒井 宏典; 神戸 振作; 仲村 愛*; 清水 悠晴*; et al.
Journal of the Physical Society of Japan, 92(5), p.053702_1 - 053702_5, 2023/05
被引用回数：2 パーセンタイル：76.59(Physics, Multidisciplinary)To investigate the static and dynamic magnetic properties on the uranium-based superconductor UTe, we measured the NMR Knight shift 
and the nuclear spin lattice relaxation rate 1/
in 
by Te-NMR on a Te-enriched single-crystal sample. 1/
in is much smaller than 1/ in 
and c, and magnetic fluctuations along each axis are derived from the 1/ measured in parallel to all three crystalline axes. The magnetic fluctuations are almost identical at two Te sites and isotropic at high temperatures, but become anisotropic below 40 K, where heavy-fermion state is formed.
-axis knight shift on UTe with 
= 2.1 K松村 拓輝*; 藤林 裕己*; 金城 克樹*; 北川 俊作*; 石田 憲二*; 徳永 陽; 酒井 宏典; 神戸 振作; 仲村 愛*; 清水 悠晴*; et al.
Journal of the Physical Society of Japan, 92(6), p.063701_1 - 063701_5, 2023/05
被引用回数：8 パーセンタイル：93.15(Physics, Multidisciplinary)Spin susceptibility in the superconducting (SC) state was measured in the higher-quality sample of uranium-based superconductor UTe by using Knight-shift measurements for a magnetic field along all three crystalline axes. In the higher-quality sample, the SC transition temperature is about 2.1 K, and the residual electronic term in the specific heat is almost zero. The NMR linewidth becomes narrower and is almost half of that in the previous sample with 
1.6 K when and 
. Although the Knight-shift behavior was not so different from the previous results for 
, and , a large reduction in Knight shift along the axis was observed, in contrast with the previous -axis Knight shift result. We discuss the origin of the difference between the previous and present results, and the possible SC state derived from the present results.
Lee, S.*; 仲田 光樹; Tchernyshyov, O.*; Kim, S. K.*
Physical Review B, 107(18), p.184432_1 - 184432_12, 2023/05
被引用回数：5 パーセンタイル：87.72(Materials Science, Multidisciplinary)超対称量子力学に基づき、反強磁性スカーミオン構造を有する磁壁中のマグノンのトポロジカル量子輸送物性を明らかにする。スカーミオン型の磁気構造を有する磁壁中を伝搬するマグノンは、一種のゲージ場として作用する有効磁場を獲得する。そこで、この有効磁場中でのマグノンの反射・屈折現象を超対称量子力学に基づいて解析し、その伝搬および束縛マグノン状態を明らかにする。そして、ラウダウアー公式を用いて、磁壁のカイラリティが増加するにつれてマグノンによる熱流が減少することを明らかにする。本研究はスピンホール効果を活用した熱流の制御方法を理論的に提案する。
山 正樹*; 松尾 衛; 加藤 岳生*
Physical Review B, 107(17), p.174414_1 - 174414_15, 2023/05
被引用回数：1 パーセンタイル：49.29(Materials Science, Multidisciplinary)We theoretically consider the effect of vertex correction on spin pumping from a ferromagnetic insulator (FI) into a two-dimensional electron gas (2DEG) in which the Rashba and Dresselhaus spin-orbit interactions coexist. The Gilbert damping in the FI is enhanced by elastic spin-flipping or magnon absorption. We show that the Gilbert damping due to elastic spin-flipping is strongly enhanced by the vertex correction when the ratio of the two spin-orbit interactions is near a special value at which the spin relaxation time diverges while that due to magnon absorption shows only small modification. We also show that the shift in the resonant frequency due to elastic spin-flipping is strongly enhanced in a similar way as the Gilbert damping.
along hard magnetic axis酒井 宏典; 常盤 欣文; Opletal, P.; 木俣 基*; 淡路 智*; 佐々木 孝彦*; 青木 大*; 神戸 振作; 徳永 陽; 芳賀 芳範
Physical Review Letters, 130(19), p.196002_1 - 196002_6, 2023/05
被引用回数：6 パーセンタイル：93.15(Physics, Multidisciplinary)
=2.1Kのウラン2テルル化物単結晶における超伝導相図を磁気困難軸である結晶軸方向に磁場をかけて調べた。電気抵抗と交流帯磁率を同時に測定した結果、低磁場超伝導(LFSC)相と高磁場超伝導(HFSC)相が、対照的な磁場-角度依存性をもつことがわかった。結晶の純良性が上がったことにより、LFSC相の上部臨界磁場は上昇したものの、HFSC相が現れる特徴磁場
は、単結晶の純良性に関わらず、15Tと一定であることがわかった。また、近傍のLFSC相内に、弱い渦糸ピン留め力で特徴づけられる中間超伝導相を示唆する新たな相線の形跡を捉えた。
増田 啓人*; 山根 結太*; 関 剛斎*; Raab, K.*; 土肥 昂尭*; Modak, R.*; 内田 健一*; 家田 淳一; Kl
ui, M.*; 高梨 弘毅
Applied Physics Letters, 122(16), p.162402_1 - 162402_7, 2023/04
被引用回数：1 パーセンタイル：49.29(Physics, Applied)We report current-induced magnetization switching in Pt/Co/Ir/Co/Pt multilayers with different Ir layer thicknesses (
), where the perpendicularly magnetized Co layers are coupled ferromagnetically or antiferromagnetically through an interlayer exchange coupling and are sandwiched by the Pt spin Hall layers. The domain structures formed during switching vary depending on the magnetization alignment, i.e., ferromagnetically coupled or antiferromagnetically coupled configuration. These results clarify the macroscopic picture of switching process for interlayer exchange-coupled systems. The local picture of the switching process is also examined by a numerical calculation based on a macrospin model, which reveals the switching dynamics triggered by dual spin-orbit torque for both antiferromagnetically and ferromagnetically coupled cases. The numerical calculation shows that the dual spin-orbit torque from the two Pt layers effectively acts on the two Co layers not only for the antiferromagnetically coupled case but also for the ferromagnetically coupled one. Our findings deepen the under- standing of the switching mechanism in a magnetic multilayer and provide an avenue to design spintronic devices with more efficient spin-orbit torque switching.
徳永 陽; 酒井 宏典; 北川 俊作*; 石田 憲二*
日本物理学会誌, 78(5), p.267 - 272, 2023/04
UTeは2018年末に超伝導になることが初めて報告されたウラン系超伝導体である。その発見の直後から実験と理論の両面での集中的な研究が開始され、40T以上の強磁場領域における磁場誘起超伝導や圧力下での多重超伝導相など、スピン三重項超伝導状態を起源とする新奇な超伝導現象が相次いで見つかっている。さらにその超伝導状態は、バルクとしてトポロジカル超伝導を実現する可能性があることが指摘され注目を集めている。本稿ではこのUTeにおいて、我々が行ってきた核磁気共鳴(NMR)法による研究について紹介する。
佐野 涼太郎*; 松尾 衛
Physical Review Letters, 130(16), p.166201_1 - 166201_7, 2023/04
被引用回数：1 パーセンタイル：0(Physics, Multidisciplinary)Recent experiments have shown an indication of a hydrodynamic magnon behavior in ultrapure ferromagnetic insulators; however, its direct observation is still lacking. Here, we derive a set of coupled hydrodynamic equations and study the thermal and spin conductivities for such a magnon fluid. We reveal the drastic breakdown of the magnonic Wiedemann-Franz law as a hallmark of the hydrodynamics regime, which will become key evidence for the experimental realization of an emergent hydrodynamic magnon behavior. Therefore, our results pave the way toward the direct observation of magnon fluids.
仲田 光樹; 鈴木 渓
Physical Review Letters, 130(9), p.096702_1 - 096702_6, 2023/03
被引用回数：3 パーセンタイル：76.59(Physics, Multidisciplinary)量子場の真空ゆらぎによって創発されるカシミア効果は、古典力学には対応物が存在しないという意味において真に量子力学的な効果である。しかし、カシミア効果はこれまでフォトン(光子)を舞台に研究されており、磁性体中でのカシミア効果、特にそのカシミアエネルギーの膜厚依存性については十分な理解は得られていない。そこで本研究では格子場の理論の観点から、磁性絶縁体中のスピン波を量子化したマグノンに着目し、マグノン量子場により創発されるカシミア効果「マグノン・カシミア効果」及びその膜厚依存性を明らかにする。更に反強磁性絶縁体だけでなくフェリ磁性絶縁体(例:YIG)においてもマグノン・カシミア効果が創発することを示し、スピントロニクス分野で中心的な役割を担うYIGがカシミア効果の工学的応用を目指すカシミアエンジニアリング分野にとっても絶好の舞台であることを明らかにする。本研究は、マグノン・カシミアエンジニアリングの基礎学理の構築に大きく貢献することが期待される。
